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Progress in hydrogen enriched hydrocarbons combustion and engine applications

Zuohua HUANG, Jinhua WANG, Erjiang HU, Chenglong TANG, Yingjia ZHANG

《能源前沿（英文）》 2014年 第8卷 第1期   页码 73-80 doi: 10.1007/s11708-013-0287-1

摘要： The paper summarized the work on hydrogen enriched hydrocarbons combustion and its application in engines. The progress and understanding on laminar burning velocity, flame instability, flame structure flame and chemical kinetics were presented. Based on fundamental combustion, both homogeneous spark-ignition engine and direct-injection spark-ignition engine fueled with natural gas-hydrogen blends were conducted and the technical route of natural gas-hydrogen combined with exhaust gas recirculation was proposed which experimentally demonstrated benefits on both thermal efficiency improvement and emissions reduction.

关键词： hydrogen enriched hydrocarbon combustion     fundamental study     engine application    

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Impact of oxygen enriched combustion on the performance of a single cylinder diesel engine

K. RAJKUMAR, P. GOVINDARAJAN

《能源前沿（英文）》 2011年 第5卷 第4期   页码 398-403 doi: 10.1007/s11708-011-0157-7

摘要： In the present experiment, a computerized single cylinder diesel engine with a data acquisition system was used to study the effects of oxygen enriched combustion technology (OECT) on the performance characteristics. The use of different levels of oxygen-enriched air was compared with respect to percentage load. Increasing the oxygen content in the air leads to faster burn rates and increases the combustibility at the same stoichiometry (oxygen-to-fuel ratio). These effects have the potential to increase the thermal efficiency and specific power output of a diesel engine. The power increases considerably with oxygen enrichment. In addition, oxygen enrichment can also be considered as a way to reduce the sudden loss in power output when the engine operates in a high load condition. Assessed high combustion temperature from the oxygen enriched combustion leads to high combustion efficiency. OECT reduces the volume of flue gases and reduces the effects of greenhouse effects. Engine tests were conducted in the above said engine for different loads and the following performance characteristics like brake power (BP), specific fuel consumption (SFC), mean effective pressure, brake thermal efficiency, mechanical efficiency, and exhaust gas temperature were studied. The objective of this paper is to address, in a systematic way, the key technical issues associated with applying OECT to single cylinder diesel engines.

关键词： oxygen enriched combustion     exhaust gas temperature     brake power (BP)     specific fuel consumption (SFC)    

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Combustion analysis of a hydrogen-diesel fuel operated DI diesel engine with exhaust gas recirculation

M. LOGANATHAN, A. VELMURUGAN, TOM PAGE, E. JAMES GUNASEKARAN, P. TAMILARASAN

《能源前沿（英文）》 2017年 第11卷 第4期   页码 568-574 doi: 10.1007/s11708-017-0461-y

摘要： The rapid depletion of fossil fuel and growing demand necessitates researchers to find alternative fuels which are clean and sustainable. The need for finding renewable, low cost and environmentally friendly fuel resources can never be understated. An efficient method of generation and storage of hydrogen will enable automotive manufacturers to introduce hydrogen fuelled engine in the market. In this paper, a conventional DI diesel engine was modified to operate as gas engine. The intake manifold of the engine was supplied with hydrogen along with recirculated exhaust gas and air. The injection rates of hydrogen were maintained at three levels with 2 L/min, 4 L/min, 6 L/min and 8 L/min and 10 L/min with an injection pressure of 2 bar. Many of the combustion parameters like heat release rate (HRR), ignition delay, combustion duration, rate of pressure rise (ROPR), cumulative heat release rate (CHR), and cyclic pressure fluctuations were measured. The HRR peak pressure decreased with the increase in EGR rate, while combustion duration increased with the EGR rate. The cyclic pressure variation also increased with the increase in EGR rate.

关键词： hydrogen     exhaust gas recirculation (EGR)     diesel     combustion     heat release rate (HRR)     combustion duration    

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Simulation of combustion in spark-ignition engine fuelled with natural gas-hydrogen blends combined with

Jie WANG, Zuohua HUANG, Bing LIU, Xibin WANG

《能源前沿（英文）》 2009年 第3卷 第2期   页码 204-211 doi: 10.1007/s11708-009-0026-9

摘要： A numerical simulation of the influence of different hydrogen fractions, excess air ratios and EGR mass fractions in a spark-ignition engine was conducted. Good agreement between the calculated and measured in-cylinder pressure traces as well as pollutant formation trends was obtained. The simulation results show that NO concentration has an exponential relationship with temperature and increases sharply as hydrogen is added. EGR introduction strongly influences the gas temperature and NO concentration in the cylinder. The difference in temperature will lead to even greater difference in NO concentration. Thus, EGR can effectively decrease NO concentration. NO concentration reaches its peak value at the excess air ratio of 1.1 regardless of EGR mass fraction. The study shows that natural gas-hydrogen blend combined with EGR can realize a stable combustion and low NO emission in a spark-ignition engine.

关键词： natural gas     hydrogen     NO     exhaust gas recirculation     numerical simulation    

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Effect of ignition timing and hydrogen fraction on combustion and emission characteristics of natural

WANG Jinhua, HUANG Zuohua, LIU Bing, ZENG Ke, YU Jinrong, JIANG Deming

《能源前沿（英文）》 2008年 第2卷 第2期   页码 194-201 doi: 10.1007/s11708-008-0035-0

摘要： An experimental study on the combustion and emission characteristics of a direct-injection spark-ignited engine fueled with natural gas/hydrogen blends under various ignition timings was conducted. The results show that ignition timing has a significant influence on engine performance, combustion and emissions. The interval between the end of fuel injection and ignition timing is a very important parameter for direct-injection natural gas engines. The turbulent flow in the combustion chamber generated by the fuel jet remains high and relative strong mixture stratification is introduced when decreasing the angle interval between the end of fuel injection and ignition timing giving fast burning rates and high thermal efficiencies. The maximum cylinder gas pressure, maximum mean gas temperature, maximum rate of pressure rise and maximum heat release rate increase with the advancing of ignition timing. However, these parameters do not vary much with hydrogen addition under specific ignition timing indicating that a small hydrogen fraction addition of less than 20% in the present experiment has little influence on combustion parameters under specific ignition timing. The exhaust HC emission decreases while the exhaust CO concentration increases with the advancing of ignition timing. In the lean combustion condition, the exhaust CO does not vary much with ignition timing. At the same ignition timing, the exhaust HC decreases with hydrogen addition while the exhaust CO and CO do not vary much with hydrogen addition. The exhaust NO increases with the advancing of ignition timing and the behavior tends to be more obvious at large ignition advance angle. The brake mean effective pressure and the effective thermal efficiency of natural gas/hydrogen mixture combustion increase compared with those of natural gas combustion when the hydrogen fraction is over 10%.
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我国氢动力船舶创新发展研究

童亮,袁裕鹏,李骁,严新平

《中国工程科学》 2022年 第24卷 第3期   页码 127-139 doi: 10.15302/J-SSCAE-2022.03.014

摘要：

航运业迅猛发展促使传统船舶的能耗与环境问题日益显现，氢动力船舶作为未来水路交通载运工具的发展方向之一将是实现水路交通领域碳达峰、碳中和目标的重要依托，因而研究我国氢动力船舶创新发展具有迫切性。本文梳理了氢动力船舶的发展现状，从氢动力船舶产业链发展态势、协同发展战略布局的视角完成了氢动力船舶产业布局研判；完成了发展氢动力船舶的技术经济可行性分析，覆盖氢和氨燃料、氢燃料电池、氢内燃机、基础设施、总拥有成本等角度；从氢气制取、氢气运输、大容量储氢、安全加氢、燃料电池、氢内燃机、多能源协同控制、氢应用安全等方面系统展开了氢动力船舶产业链关键环节分析。立足国情提出了我国氢动力船舶多阶段发展目标，论证形成了氢动力船舶发展路线图、氢燃料供应体系建设路径。研究建议，明晰应用场景、突破关键技术、完善配套设施、创新运营体系，以此推动我国氢动力船舶快速优质发展。

关键词： 船舶；氢动力；氢能；燃料电池；内燃机；氢燃料供应体系    

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Performance, emission and combustion characteristics of CI engine fuelled with diesel and hydrogen

R. Senthil KUMAR,M. LOGANATHAN,E. James GUNASEKARAN

《能源前沿（英文）》 2015年 第9卷 第4期   页码 486-494 doi: 10.1007/s11708-015-0368-4

摘要： Hydrogen (H ) is being considered as a primary automotive fuel and as a replacement for conventional fuels. Some of the desirable properties, like high flame velocity, high calorific value motivate us to use hydrogen fuel as a dual fuel mode in diesel engine. In this experiment, hydrogen was inducted in the inlet manifold with intake air. The experiments were conducted on a four stroke, single cylinder, water cooled, direct injection (DI), diesel engine at a speed of 1500 r/min. Hydrogen was stored in a high pressure cylinder and supplied to the inlet manifold through a water-and-air-based flame arrestor. A pressure regulator was used to reduce the cylinder pressure from 140 bar to 2 bar. The hydrogen was inducted with a volume flow rate of 4l pm, 6l pm and 8l pm, respectively by a digital volume flow meter. The engine performance, emission and combustion parameters were analyzed at various flow rates of hydrogen and compared with diesel fuel operation. The brake thermal efficiency (BTE) was increased and brake specific fuel consumption (BSFC) decreased for the hydrogen flow rate of 8l pm as compared to the diesel and lower volume flow rates of hydrogen. The hydrocarbon (HC) and carbon monoxide (CO) were decreased and the oxides of nitrogen (NO ) increased for higher volume flow rates of hydrogen compared to diesel and lower volume flow rates of hydrogen. The heat release rate and cylinder pressure was increased for higher volume flow rates of hydrogen compared to diesel and lower volume flow rates of hydrogen.

关键词： hydrogen     brake thermal efficiency     crank angle     compressed ignition (CI)    

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Activity and characteristics of “Oxygen-enriched” highly reactive absorbent for simultaneous flue gas

Yi ZHAO,Tianxiang GUO,Zili ZANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第2期   页码 222-229 doi: 10.1007/s11783-014-0636-2

摘要： An “Oxygen-enriched” highly reactive absorbent was prepared by mixing fly ash, lime and a small quantity of KMnO for simultaneous desulfurization and denitrification. Removal of SO and NO simultaneously was carried out using this absorbent in a flue gas circulating fluidized bed (CFB). The highest simultaneous removal efficiency, 94.5% of SO and 64.2% of NO, was achieved under the optimal experiment conditions. Scanning Electron Microscope (SEM) and Accessory X-ray Energy Spectrometer (EDX) were used to observe the surface characteristics of fly ash, lime, “Oxygen-enriched” highly reactive absorbent and the spent absorbent. An ion chromatograph (IC) and chemical analysis methods were used to determine the contents of sulfate, sulfite, nitrate and nitrite in the spent absorbents, the results showed that sulfate and nitrite were the main products for desulfurization and denitrification respectively. The mechanism of removing SO and NO simultaneously was proposed based on the analysis results of SEM, EDX, IC and the chemical analysis methods.

关键词： “Oxygen-enriched” highly reactive absorbent     Surface characteristics     Flue gas circulating fluidized bed     Simultaneous desulfurization and denitrification    

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氢燃料电池——重型车辆内燃发动机的替代者

Kevin Kendall, 叶思宇, 刘志祥

《工程（英文）》 2023年 第21卷 第2期   页码 39-41 doi: 10.1016/j.eng.2022.11.007

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Investigation of polyhydroxyalkanoates (PHAs) biosynthesis from mixed culture enriched by valerate-dominant

Jiuxiao Hao, Xiujin Wang, Hui Wang

《环境科学与工程前沿（英文）》 2017年 第11卷 第1期 doi: 10.1007/s11783-017-0896-8

摘要： Valerate-hydrolysate enriched culture showed great ability to produce 3HV and 3H2MV. Valerate-hydrolysate enriched culture had more in the community. Mixed iso-/n-valerate was effective at balancing microbial growth and PHAs synthesis. Co-substrates of valerate and propionate raised the fraction of 3HV and 3H2MV. The production of polyhydroxyalkanoates (PHAs) with a high fraction of 3-hydroxyvalerate (3HV) and 3-hydroxy-2-methylvalerate (3H2MV) from mixed culture enriched by valerate-dominant hydrolysate was evaluated in this study. After long-term enrichment, the culture showed strong ability to synthesize 3HV and 3H2MV, even with acetate-dominant substrate. The ultilization of single or mixed iso-/n-valerate by the enriched culture showed that the mixture of iso-valerate and n-valerate was more efficient substrate than any single in terms of balancing microbial growth and PHAs synthesis. Besides, through comparing the kinetics and stoichiometry of the tests supplying valerate and propionate, the enriched culture with equivalent valerate and propionate (1:1 molar ratio) exhibited superior PHAs production performances to pure valerate or propionate, attaining more than 70 mol% of 3HV and 3H2MV. The above findings reveal that valerate-dominant hydrolysate is a kind of suitable substrate to enrich PHAs producing culture with great capability to synthesize 3HV and 3H2MV monomers, thus improving product properties than pure poly(3-hydroxybutyrate) (P3HB); also 3HV and 3H2MV production behaviors can be regulated by the type of odd-carbon VFAs in the substrate.

关键词： Polyhydroxyalkanoates (PHAs)     Valerate     Mixed culture     3-hydroxyvalerate (3HV)     Propionate    

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中国古生代海相油气成藏特征

康玉柱

《中国工程科学》 2010年 第12卷 第5期   页码 11-17

摘要：

1970―1978年笔者在塔里木油气地质调研中首次提出古生代有发育的烃源岩，1984年沙参2井实现了古生代海相油田的首次重大突破。1992年通过多个古生代油气田深入研究建立了古生代海相油气成藏理论。其理论内涵：叠加复合盆地成藏，多时代多层系生油，多期成藏，多时代多类型储盖组合，多成藏模式，油气主要分布在古隆起、古斜坡、断裂带和不整合面附近。

关键词： 古生代     海相油气田     盆地     隆起     坳陷     油气分布    

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exogenous degrader-enhanced bioremediation with low-dose persulfate oxidation for polycyclic aromatic hydrocarbon

《环境科学与工程前沿（英文）》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1733-x

摘要： Polycyclic aromatic hydrocarbon (PAH)-contaminated soils are usually complex and characterized by a lack of nutrition and soil salinization, resulting in difficulties in soil remediation. In this study, bioaugmentation with a PAH-degrading Bacillus PheN7 (BA) and low-dose persulfate oxidation (PS), along with natural biodegradation, were utilized to remediate alkaline PAH-contaminated soil. The soil used in the study had a pH of 9.35, and the total PAH content was 568.8 ± 31.0 mg/kg dry soil. After 42 d of remediation, the degradation efficiency of PAHs was 96.72% and 93.88% using persulfate oxidation and bioaugmentation, respectively, whereas 38.66% of PAHs were degraded in natural attenuation (NA). Bacillus was the dominant genera throughout the process of bioremediation with the relative abundance of 79.3% on day 42 in the BA system, whereas, Alcanivorax was enriched and became the dominant genera in PS systems. In the meantime, PAH degradation genes were detected with remarkably higher level in the BA system than in PS system during the remediation. In addition to the degradation of contaminants, persulfate oxidation promotes microbial bioremediation efficiency mainly by lowering the pH to neutral and increasing the active phosphorus content in the soil. Microbial species and ecological niches were less reduced in the PS system than in the BA system. Collectively, persulfate oxidation had a better impact on the soil microbiome and is more suitable for long-term soil health than bioaugmentation through PheN7 addition.

关键词： Bioaugmentation     Low-dose persulfate oxidation     Polycyclic aromatic hydrocarbon     Remediation    

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Adsorption of phosphate on magnetite-enriched particles (MEP) separated from the mill scale

Muhammad Kashif Shahid, Yunjung Kim, Young-Gyun Choi

《环境科学与工程前沿（英文）》 2019年 第13卷 第5期 doi: 10.1007/s11783-019-1151-2

摘要： MEP were separated from mill scale at low magnetic intensity i.e., 300 to 500 gauss. The phosphate adsorption capacity of MEP was determined 6.41 mg/g. MEP packed-bed columns were successfully regenerated with alkaline solution. Phosphate is a major pollutant in water, causing serious environmental and health consequences. In present study, the phosphate adsorption on novel magnetite-enriched particles (MEP) was comprehensively investigated. A new method and device were introduced for the separation of MEP from the mill scale at low magnetic intensity. Particles were characterized with different techniques such as XRD, XRF, SEM and EDS. The XRD and XRF analysis of MEP identified the dominant existence of crystalline magnetite. Furthermore, the morphological analysis of MEP confirmed the agglomerate porous morphology of magnetite. Oxygen and iron, the main constituents of magnetite were acknowledged during the elemental analysis using EDS. The phosphate adsorption on MEP is well explained using various isotherm and kinetic models, exhibiting the monolayer adsorption of phosphate on the surface of MEP. The maximum adsorption capacity was determined 6.41 mg/g. Based on particle size (45–75 and 75–150 µm) and empty bed contact time (1 and 2 h), four columns were operated for 54 days. MEP were appeared successful to remove all phosphate concentration from the column influent having 2 mg/L concentration. The operated column reactors were successfully regenerated with alkaline solution. The results indicated potential for practical application of the MEP for phosphate removal.

关键词： Adsorption     Magnetite     Mill-scale     Phosphate     Wastewater treatment    

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中国非常规油气的潜力和发展

胡文瑞,翟光明,李景明

《中国工程科学》 2010年 第12卷 第5期   页码 25-29

摘要：

概述了国外和我国非常规油气资源开发利用状况，分析了我国发展非常规油气存在的困难，提出了加快发展我国非常规油气的对策与建议。

关键词： 非常规油气     勘探开发     技术     潜力     对策    

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Anaerobic phenanthrene biodegradation with four kinds of electron acceptors enriched from the same mixed

Zuotao Zhang, Chongyang Wang, Jianzhong He, Hui Wang

《环境科学与工程前沿（英文）》 2019年 第13卷 第5期 doi: 10.1007/s11783-019-1164-x

摘要： Anaerobic phenanthrene biodegradation enriched process was described in detail. The enriched bacterial communities were characterized under four redox conditions. The enriched archaeal communities were stated under high percentage conditions. Relatively intact pathways of anaerobic phenanthrene biodegradation were proposed. Polycyclic aromatic hydrocarbons (PAHs) are widespread and persistent contaminants worldwide, especially in environments devoid of molecular oxygen. For lack of molecular oxygen, researchers enhanced anaerobic zones PAHs biodegradation by adding sulfate, bicarbonate, nitrate, and iron. However, microbial community reports of them were limited, and information of metabolites was poor except two-ring PAH, naphthalene. Here, we reported on four phenanthrene-degrading enrichment cultures with sulfate, bicarbonate, nitrate, and iron as electron acceptors from the same initial inoculum. The high-to-low order of the anaerobic phenanthrene biodegradation rate was the nitrate-reducing conditions>sulfate-reducing conditions>methanogenic conditions>iron-reducing conditions. The dominant bacteria populations were Desulfobacteraceae, Anaerolinaceae, and Thermodesulfobiaceae under sulfate-reducing conditions; Moraxellaceae, Clostridiaceae, and Comamonadaceae under methanogenic conditions; Rhodobacteraceae, Planococcaceae, and Xanthomonadaceae under nitrate-reducing conditions; and Geobacteraceae, Carnobacteriaceae, and Anaerolinaceae under iron-reducing conditions, respectively. Principal component analysis (PCA) indicated that bacteria populations of longtime enriched cultures with four electron acceptors all obtained significant changes from original inoculum, and bacterial communities were similar under nitrate-reducing and iron-reducing conditions. Archaea accounted for a high percentage under iron-reducing and methanogenic conditions, and Methanosarcinaceae and Methanobacteriaceae, as well as Methanobacteriaceae, were the dominant archaea populations under iron-reducing and methanogenic conditions. The key steps of phenanthrene biodegradation under four reducing conditions were carboxylation, further ring system reduction, and ring cleavage.

关键词： Phenanthrene     Anaerobic biodegradation     Bacterial populations     Archaea populations     Metabolic pathway    

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标题 作者 时间 类型 操作

Progress in hydrogen enriched hydrocarbons combustion and engine applications

Zuohua HUANG, Jinhua WANG, Erjiang HU, Chenglong TANG, Yingjia ZHANG

期刊论文

Impact of oxygen enriched combustion on the performance of a single cylinder diesel engine

K. RAJKUMAR, P. GOVINDARAJAN

期刊论文

Combustion analysis of a hydrogen-diesel fuel operated DI diesel engine with exhaust gas recirculation

M. LOGANATHAN, A. VELMURUGAN, TOM PAGE, E. JAMES GUNASEKARAN, P. TAMILARASAN

期刊论文

Simulation of combustion in spark-ignition engine fuelled with natural gas-hydrogen blends combined with

Jie WANG, Zuohua HUANG, Bing LIU, Xibin WANG

期刊论文

Effect of ignition timing and hydrogen fraction on combustion and emission characteristics of natural

WANG Jinhua, HUANG Zuohua, LIU Bing, ZENG Ke, YU Jinrong, JIANG Deming

期刊论文

我国氢动力船舶创新发展研究

童亮,袁裕鹏,李骁,严新平

期刊论文

Performance, emission and combustion characteristics of CI engine fuelled with diesel and hydrogen

R. Senthil KUMAR,M. LOGANATHAN,E. James GUNASEKARAN

期刊论文

Activity and characteristics of “Oxygen-enriched” highly reactive absorbent for simultaneous flue gas

Yi ZHAO,Tianxiang GUO,Zili ZANG

期刊论文

氢燃料电池——重型车辆内燃发动机的替代者

Kevin Kendall, 叶思宇, 刘志祥

期刊论文

Investigation of polyhydroxyalkanoates (PHAs) biosynthesis from mixed culture enriched by valerate-dominant

Jiuxiao Hao, Xiujin Wang, Hui Wang

期刊论文

中国古生代海相油气成藏特征

康玉柱

期刊论文

exogenous degrader-enhanced bioremediation with low-dose persulfate oxidation for polycyclic aromatic hydrocarbon

期刊论文

Adsorption of phosphate on magnetite-enriched particles (MEP) separated from the mill scale

Muhammad Kashif Shahid, Yunjung Kim, Young-Gyun Choi

期刊论文

中国非常规油气的潜力和发展

胡文瑞,翟光明,李景明

期刊论文

Anaerobic phenanthrene biodegradation with four kinds of electron acceptors enriched from the same mixed

Zuotao Zhang, Chongyang Wang, Jianzhong He, Hui Wang

期刊论文